Publication detail

Recent Advances on Heteroatom-Doped Porous Carbon—Based Electrocatalysts for Oxygen Reduction Reaction

Li, Xue Liu, Guolei Zheng, Han Sun, Kuizhao Wan, Linna Cao, Jing Asif, Saira Cao, Yue Si, Weimeng Wang, Fagang Bokhari, Awais

English title

Recent Advances on Heteroatom-Doped Porous Carbon—Based Electrocatalysts for Oxygen Reduction Reaction

Type

journal article in Web of Science

Language

en

Original abstract

Polymer electrolyte membrane fuel cells are considered one of the alternatives to fossil energy sources. The slow kinetics of the oxygen reduction reaction (ORR) at the cathode and the high price of Pt-based catalysts remain one of the key challenges for the commercial viability of proton exchange membrane fuel cells. However, their high cost and susceptibility to poisoning severely limit their use for large-scale commercial applications in fuel cells. Heteroatom-doped porous carbon has attracted extensive attention from scientists due to its advantages such as high specific surface area and the properties conferred by heteroatom doping. On the one hand, we discuss a variety of current methods for the preparation of heteroatom-doped porous carbons, including the template method and the activation method. On the other hand, we discuss the application of heteroatom-doped porous carbon in Pt catalysts, transition metal catalysts and metal-free catalysts. Finally, we also present the pre-existing and challenges of heteroatoms in ORR catalysis, which will drive the development of ORR catalysts.

English abstract

Polymer electrolyte membrane fuel cells are considered one of the alternatives to fossil energy sources. The slow kinetics of the oxygen reduction reaction (ORR) at the cathode and the high price of Pt-based catalysts remain one of the key challenges for the commercial viability of proton exchange membrane fuel cells. However, their high cost and susceptibility to poisoning severely limit their use for large-scale commercial applications in fuel cells. Heteroatom-doped porous carbon has attracted extensive attention from scientists due to its advantages such as high specific surface area and the properties conferred by heteroatom doping. On the one hand, we discuss a variety of current methods for the preparation of heteroatom-doped porous carbons, including the template method and the activation method. On the other hand, we discuss the application of heteroatom-doped porous carbon in Pt catalysts, transition metal catalysts and metal-free catalysts. Finally, we also present the pre-existing and challenges of heteroatoms in ORR catalysis, which will drive the development of ORR catalysts.

Keywords in English

catalyst; heteroatom doping; oxygen reduction; platinum; porous carbon; specific surface area; transition metal

Released

21.01.2023

Publisher

MDPIST ALBAN-ANLAGE 66, CH-4052 BASEL, SWITZERLAND

Location

MDPIST ALBAN-ANLAGE 66, CH-4052 BASEL, SWITZERLAND

ISSN

1996-1073

Volume

1

Number

16

Pages count

15

BIBTEX


@article{BUT187700,
  author="Saira {Asif} and Šárka {Zemanová} and Syed Awais Ali Shah {Bokhari},
  title="Recent Advances on Heteroatom-Doped Porous Carbon—Based Electrocatalysts for Oxygen Reduction Reaction",
  year="2023",
  volume="1",
  number="16",
  month="January",
  publisher="MDPIST ALBAN-ANLAGE 66, CH-4052 BASEL, SWITZERLAND",
  address="MDPIST ALBAN-ANLAGE 66, CH-4052 BASEL, SWITZERLAND",
  issn="1996-1073"
}